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COMMUNICATION
Journal Name
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4 Y. Li, S. Huang, Z. Cheng, K. Cai, L. Li, E. Milan, J. Lv, Y. Wang, Q. Sun
specially adapted for synthesizing SUZ-4, but it is difficult to be
+
and X. Ma, Appl. Catal. B Environ., 2019, 256, 1I:17777.
DO 10.1039/D0CC00886A
fully ion-exchanged because a substantial amount of K located
5 M. Boronat, C. Martinez-Sanchez, D. Law and A. Corma, J. Am. Chem.
Soc., 2008, 130, 16316-16323.
6 X. Feng, J. Yao, H. Li, Y. Fang, Y. Yoneyama, G. Yang and N. Tsubaki,
Chem. Commun., 2019, 55, 1048-1051.
7 S. L. Lawton, J. M. Bennett, J. L. Schlenker and M. K. Rubin, J. Chem.
Soc. Chem. Commun., 1993, 11, 894-896.
8 K. G. Strohmaier, M. Afeworki and D. L. Dorset, Z. Kristallogr., 2006,
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7,29,45
in the small cages and/or the double six-member rings.
The K/Al ratio was 0.296 on the HSUZ-4 catalyst discussed
above, and it was reduced to 0.132 by using an intensive ion-
exchange procedure. As a result, the conversion of DME
0
enhanced from 22% to 26% at 220 C (Fig. S10).
In summary, HSUZ-4 constituted a new type of zeolite catalyst
for DME carbonylation with superior performance to HZSM-35
that have quite similar acid features and pore structures. Most
likely, the abundant 8-MR pore openings on the rod-shaped
HSUZ-4 facilitated the diffusion of the reactive molecules.
We gratefully acknowledge the National Natural Science
Foundation of China (21773229)
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21, 689-698.
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Conflicts of interest
There are no conflicts to declare.
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5 Z. Ma and J. A. van Bokhoven, ChemCatChem, 2012, 4, 2036-2044.
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